OK, we'll get technical. Yes, you'll want a PCI-E. Be sure to not get it in PCI (even though the 6600GT was never made in PCI) and only look for PCI-E.
Technically, the PCI-E version is 29x faster than the PCI version that never existed, not 100x.
Regardless, the 6600GT is a good cheap alternative if you are on a tight budget and want to buy some time to save up for a better card.
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